Non-equilibrium Thermodynamics of Heterogeneous Systems. Signe Kjelstrup

Non-equilibrium Thermodynamics of Heterogeneous Systems - Signe Kjelstrup


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18.5Thermal osmosis

       19Modeling the polymer electrolyte fuel cell

       19.1The potential work of a fuel cell

       19.2The cell and its five subsystems

       19.3The electrode backing and the membrane

       19.3.1The entropy production in the homogeneous phases

       19.3.2The anode backing

       19.3.3The membrane

       19.3.4The cathode backing

       19.4The electrode surfaces

       19.4.1The anode catalyst surface

       19.4.2The cathode catalyst surface

       19.5A model in agreement with the second law

       19.6Concluding comments

       20Measuring membrane transport properties

       20.1The membrane in equilibrium with electrolyte solutions

       20.2The membrane resistivity

       20.3Ionic transport numbers

       20.4The transference number of water and the water permeability

       20.5The Seebeck coefficient

       20.6Interdiffusion coefficients

       21The impedance of an electrode surface

       21.1The hydrogen electrode: Mass balances

       21.2The oscillating field

       21.3Reaction Gibbs energies

       21.4The electrode surface impedance

       21.4.1The adsorption–diffusion layer in front of the catalyst

       21.4.2The charge transfer reaction

       21.4.3The impedance spectrum

       21.5A test of the model

       21.6The reaction over potential

       22Non-equilibrium molecular dynamics simulations

       22.1The system

       22.1.1The interaction potential

       22.2Calculation techniques

       22.3Verifying the assumption of local equilibrium

       22.3.1Local equilibrium in a homogeneous binary mixture

       22.3.2Local equilibrium in a gas–liquid interface

       22.4Verifications of the Onsager relations

       22.4.1A homogeneous binary mixture

       22.4.2Agas–liquidinterface

       22.5Linearity of the flux–force relations

       22.6Molecular mechanisms

       23The non-equilibrium two-phase van der Waals model

       23.1Van der Waals equation of states

       23.2Van der Waals square gradient model for the interfacial region

       23.3Balance equations

       23.4The entropy production

       23.5Flux equations

       23.6A numerical solution method

       23.7Procedure for extrapolation of bulk densities and fluxes

       23.8Defining excess densities

       23.9Thermodynamic properties of Gibbs’ surface

       23.10An autonomous surface

       23.11Excess


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